In article number 1903142, Ayumi Ishii and Tsutomu Miyasaka demonstrate near-infrared light emitting diodes based on an energy transfer from wide bandgap all inorganic perovskite to ytterbium ions as an emitter in the crystalline film. The high light-emitting efficiency around 1000 nm in the perovskite-based diodes provides a new possibility for future optical applications.