Identification of the conductivity type of single-walled carbon nanotubes via dual-modulation dielectric force microscopy

材料科学 欧姆接触 碳纳米管 电导率 光电子学 电压 载流子 整改 半导体 电介质 栅极电介质 晶体管 纳米技术 电气工程 化学 图层(电子) 物理化学 工程类
作者
Junqi Lai,Wenyuan Wang,Z. Liu,Bowen Chen,Lixing Kang,Qi Chen,Liwei Chen
出处
期刊:Journal of Chemical Physics [American Institute of Physics]
卷期号:161 (3)
标识
DOI:10.1063/5.0205512
摘要

The conductivity type is one of the most fundamental transport properties of semiconductors, which is usually identified by fabricating the field-effect transistor, the Hall-effect device, etc. However, it is challenging to obtain an Ohmic contact if the sample is down to nanometer-scale because of the small size and intrinsic heterogeneity. Noncontact dielectric force microscopy (DFM) can identify the conductivity type of the sample by applying a DC gate voltage to the tip, which is effective in tuning the accumulation or depletion of charge carriers. Here, we further developed a dual-modulation DFM, which simplified the conductivity type identification from multiple scan times under different DC gate voltages to a single scan under an AC gate voltage. Taking single-walled carbon nanotubes as testing samples, the semiconducting-type sample exhibits a more significant charge carrier accumulation/depletion under each half-period of the AC gate voltage than the metallic-type sample due to the stronger rectification effect. The charge carrier accumulation or depletion of the p-type sample is opposite to that of the n-type sample at the same half-period of the AC gate voltage because of the reversed charge carrier type.

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