Bioinspired artificial luminescent skin (L-skin) integrated with multiple sensing functions significantly promotes the development of smart devices. It is considerably challenging to realize underwater sensing technologies. Here, a sharkskin-inspired Eu@HOF-TJ-1@TA L-skin (1) is prepared for both temperature and sound sensing. 1 is an ultrathin and flexible temperature sensor, in 298.15-358.15 K, exhibiting ultrahigh maximum relative sensitivity (97.669% K