电容去离子
石墨烯
材料科学
多孔性
化学工程
氮气
吸附
纳米技术
大孔隙
兴奋剂
多孔介质
碳纤维
微型多孔材料
水溶液
石墨烯泡沫
复合材料
介孔材料
电化学
氧化石墨烯纸
复合数
化学
光电子学
有机化学
电极
催化作用
物理化学
工程类
作者
Owen Noonan,Yueqi Kong,Yang Liu,Mohammed Kalantari,Nanjundan Ashok Kumar,Xiaodan Huang,Chengzhong Yu
标识
DOI:10.1002/aesr.202100190
摘要
Graphene foam materials have attracted particular attention for capacitive deionization (CDI) applications due to their robust conductive framework and open three‐dimensional porous structures. However, their salt adsorption capacities (SACs) are limited by the bland macropores and poor compatibility with aqueous environments. Herein, hierarchical porous nitrogen‐doped spray‐dried graphene (N‐SDG) is prepared through a spray‐drying method followed by low‐temperature nitrogen doping. The resulting material exhibits hierarchical porosity and a nitrogen‐rich carbon framework which demonstrates an improved SAC of 19.6 mg g −1 in 500 mg L −1 NaCl solution, amongst the highest reported for graphene‐based CDI materials. The method herein demonstrates a commercially attractive approach for the production of N‐doped porous graphene material for CDI applications. These findings are expected to underpin new developments in low‐cost graphene‐based materials for a range of applications.
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