自发辐射
光致发光
离子
塞尔效应
材料科学
光电子学
吸收(声学)
辐射传输
发光
光子学
色散(光学)
格子(音乐)
电介质
激发
激子
光学
分子物理学
原子物理学
指向性
光发射
光子晶体
热光电伏打
物理
纳米光子学
发射光谱
受激发射
厚板
可见光谱
荧光
等离子体子
表面等离子体子
超辐射
切伦科夫辐射
作者
Zhuang Li,Shuizhu Yu,Xianyu Ao
标识
DOI:10.1021/acsphotonics.6c01542
摘要
Abstract Rare-earth ions are pivotal for integrated photonic light sources, but their low optical transition cross sections inherently limit pump absorption efficiency and spontaneous emission rates. Here, we overcome these drawbacks by designing a dielectric metasurface that supports dual flat bands, which synergistically enhance both excitation and emission processes. Strong momentum–space anticrossings arise from hybridization between transverse-electric-like and transverse-magnetic-like surface lattice resonances hosted by a TiO2 nanodisk array integrated on a Yb3+-doped Ta2O5 slab waveguide, giving rise to two spectrally separated flat bands. The shorter-wavelength flat band resonantly boosts pump absorption, whereas the longer-wavelength counterpart elevates the radiative decay rate of emitters through the Purcell effect. Angle-resolved measurements corroborate the dispersion characteristics of these flat bands. Under resonant excitation, we demonstrate a photoluminescence enhancement of over 250-fold, alongside a marked reduction in emission lifetime from 0.47 to 0.1 ms. Back-focal-plane imaging further confirms that the boosted luminescence aligns with the pre-engineered flat-band dispersion relation. This scheme offers a general route to tailor pump absorption efficiency, radiative decay rate, and emission directivity toward high-performance rare-earth-ion-based on-chip light sources.
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