佩多:嘘
材料科学
生物传感器
复合数
纳米技术
可穿戴计算机
电极
纳米纤维
适体
导电聚合物
光电子学
计算机科学
聚合物
化学
复合材料
嵌入式系统
图层(电子)
物理化学
生物
遗传学
作者
Yutong Shen,Shan-Shan Chai,Qingling Zhang,Mengdi Zhang,Xue Mao,Lubin Wei,Fenglei Zhou,Runjun Sun,Chengkun Liu
标识
DOI:10.1016/j.cej.2023.146008
摘要
The detection of lactate and other bioactive molecules is of great significance in biological research, medical testing, and environmental monitoring. Organic electrochemical transistors are a kind of biosensor devices, which can convert biological signals into electrical signals. In recent years, fiber-based organic electrochemical transistors (FECTs) provide a new approach for the construction of flexible wearable biosensors, promoting greatly the development of flexible wearable electronic products. In this study, a multilayer composite electrode was first prepared by incorporating MXene and PEDOT:PSS onto electrospun oriented polyvinyl formal (PVF) nanofiber bundle, and then assembled into FECT with high sensitivity and selectivity. Meanwhile, a wearable real-time monitoring platform was built to detect the lactate concentrations in human sweat. The results showed that MXene could act as a bridge between PEDOT:PSS and PVF, and the sensing performance of PVF/MXene/PEDOT:PSS-based FECT was enhanced obviously. It had a wide linear response range of 1 nM-100 mM, a sensitivity of 0.442 NCR/decade, a quick response time of 0.5 s, a low detection concentration, an excellent reproducibility, and a superior anti-interference characteristic. Therefore, this work provided more possibilities for the development of wearable biosensor.
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