扫描流动性粒度仪
粒子数
环境科学
粒子(生态学)
相对湿度
大气科学
水槽(地理)
气溶胶
粒度分布
空气质量指数
粒径
云凝聚核
体积热力学
成核
气象学
化学
地理
物理
热力学
地质学
物理化学
海洋学
有机化学
地图学
作者
Jing Wang,Mengren Li,Lingjun Li,Ronghua Zheng,Xiaolong Fan,Youwei Hong,Lingling Xu,Jinsheng Chen,Baoye Hu
标识
DOI:10.1016/j.scitotenv.2022.154208
摘要
New particle formation (NPF) has a great impact on regional and global climate, air quality and human health. This study uses a Scanning Mobility Particle Sizer (SMPS) for simultaneous measurement of particle number size distribution (PNSD) in wintertime to investigate NPF in the coastal city of Xiamen. The mean particle number concentration, surface area concentration and volume concentration were 7.25 × 10 3 cm −3 , 152.54 μm 2 cm −3 , and 4.03 μm 3 cm −3 , respectively. Particle number concentration was mainly influenced by the nucleation mode and the Aitken mode, whereas the main contributor to particle surface area concentration and volume concentration was accumulation mode particles. The frequency of NPF events occurred was around 41.4% in December 2019. The typical growth rates of new formed particles were 1.41–2.54 nm h −1 , and the observed formation rates were 0.49–1.43 cm −3 s −1 . A comparative analysis of conditions between event and non-event days was performed. The results emphasized that air temperature, UV radiation and relative humidity were the most decisive meteorological factors, and NPF events usually occurred under clean atmospheric conditions with low PM concentrations. Although condensation sink was high when NPF event occurred, the level of SO 2 and O 3 concentration was also high. • Aitken mode particle contributed about 50% of the particle number concentration. • High frequency of NPF events was observed in the coastal city Xiamen. • NPF events mainly showed ‘banana’ shape in Xiamen wintertime. • NPF events occurred with high temperature, high radiation, and low relative humidity.
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