量子点
超声
剥脱关节
碳化
光致发光
材料科学
荧光
溶剂
碳量子点
吸收(声学)
碳纤维
纳米技术
发光
化学工程
光化学
光电子学
化学
有机化学
光学
扫描电子显微镜
复合数
复合材料
石墨烯
物理
工程类
作者
Weimin Zhang,Jinhong Du,Zhibo Liu,Dingdong Zhang,Qinwei Wei,Haichao Liu,Wei Ma,Wencai Ren,Hui‐Ming Cheng
出处
期刊:Carbon
[Elsevier]
日期:2019-12-01
卷期号:155: 243-249
被引量:11
标识
DOI:10.1016/j.carbon.2019.08.067
摘要
N-methyl-2-pyrrolidone (NMP) has been widely used as a solvent for preparing two-dimensional quantum dots (2D-QDs) by probe sonication. Here we found that carbon dots (CDs) are simultaneously produced by the carbonization of NMP when preparing MoS2 QDs in a NMP solvent by probe sonication. These two kinds of QDs are similar in color, crystal structure, excitation wavelength dependent photoluminescence (PL), and have overlaps in their absorption spectra and coincidence of PL peaks. As a result, the co-production of CDs has not previously been recognized. The CDs show strong optical interactions with the MoS2 QDs, which leads to a dramatic decrease in the fluorescence intensity of the CDs/MoS2 QDs. Moreover, we found that the carbonization also occurs for the commonly used organic solvents. These findings suggest that associated production of CDs should be considered when preparing 2D-QDs by probe sonication, and the resulting hybrid CDs/2D-QDs will provide opportunities to design their properties and uses.
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