Rapid population and economic growth intensify carbon emissions and degrade land carbon sinks. While existing research predominantly focuses on urban energy emissions, systematic studies addressing comprehensive land-carbon interactions in China’s key urban agglomerations remain lacking. This research integrates Markov-FLUS and extended STIRPAT models to simulate 2021–2040 land-use and carbon emissions in the Guangdong-Hong Kong-Macao Greater Bay Area (GBA) under low-carbon, moderate, and extensive development scenarios. Key findings: The moderate development scenario achieves the most balanced land-use changes, whereas other scenarios exhibit extreme shifts in specific land types. Significant land-use transformations predominantly occur in ecologically sensitive areas across all scenarios, particularly in peri -urban zones and administrative boundaries. The GBA will achieve carbon peaking by 2030 under low-carbon (470.3 million tons) and moderate scenarios (520.1 million tons), but experience 1 year postponement under extensive development scenario (563.3 million tons). Cities are categorized into 4 groups based on their peaking timelines and emission levels. Land-based carbon sequestration remains substantially lower than emissions throughout the region (less than 5 %). Therefore, the core of decarbonization development in the GBA resides in controlling carbon source emissions. Achieving low-carbon and sustainable development in the GBA requires comprehensive consideration of land circulation changes and green urban development.