Commercial pure titanium sheet was rolled by means of asymmetric rolling in order to obtain nanocrystallines in the top-surface layer, the microstructural evolution was examined by using different experimental techniques.Experimental results show that, after the asymmetric rolling, equiaxed nanocrystallines of about 30-60 nm in size form in the top-surface layer of sheet.The research work indicates that the surface nanocrystallization can be realized for large-dimensional metal sheets during the rolling process by using the asymmetric rolling.The asymmetric rolling induced surface nanocrystallization mechanism was summarized as follows: upon the application of repeated loads, dislocation cells/sub-micro-grains form through slips, annihilations and recombinations of high density of dislocations; with the increment of rolling pass and reduction, high density of dislocations in the refined cells/grains developing in above route lead to the reduction of grain size and the increment of misorientations between the refined grains, and finally * ÁÝÅ´