催化作用
串联
分区(防火)
同种类的
化学
组合化学
纳米技术
均相催化
多相催化
材料科学
有机化学
物理
热力学
复合材料
酶
作者
Tania Rodenas,Gonzalo Prieto
标识
DOI:10.1002/cctc.202201058
摘要
Tandem catalysis stands out as a major instrument towards the intensification of existing and future chemical processes. Initially formulated in the field of homogeneous catalysis, the concept relies on the single-pot integration of two (or more) catalysts showing high specificity for mechanistically decoupled reactions, while being operational and compatible under a single set of operation conditions. Isolated metal atoms stabilized on solid carriers in single-atom catalysts (SACs) hold the potential to reconcile the high reaction specificities of mononuclear sites in molecular catalysts with an intrinsic catalyst compartmentalization on inorganic matrices. Understandably, SACs have started to be considered as platforms in tandem catalysis. Tandem (electro)catalytic processes based on SACs have been showcased recently. While this sets excellent prospects for the expansion of this research subarea, challenges are faced, particularly as to the verification of the tandem nature of the processes.
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