电催化剂
纳米技术
塔菲尔方程
化学
纳米材料
分解水
纳米颗粒
合金
电解
电子转移
量子点
电解水
催化作用
材料科学
电解质
电化学
电极
有机化学
物理化学
光催化
作者
Farooq Sher,Imane Ziani,Maren L. Smith,Galina N. Chugreeva,Seyid Zeynab Hashimzada,Liziê Daniela Tentler Prola,Jasmina Sulejmanović,Emina Karahmet Sher
标识
DOI:10.1016/j.ccr.2023.215499
摘要
The recent advances in nanomaterials have led to speculation about the effectivity of carbon quantum dots applied as electrocatalysts for water splitting. An insufficient amount of research has been undergone into this proposed application, although CQDs exhibit great potential with rapid electron transfer rates, long-term stability and desirable morphologies. To evaluate various materials that could aid CQDs in their application as electrocatalysts for water splitting, investigate environmentally conscious synthesis routes and determine whether the application could be considered for commercial applications, numerous studies and articles were collated to obtain a comprehensive strategy for processing and analysing data. Further, investigating not only CQDs but metal alloy nanoparticles, along with their current uses and the other supporting materials they have been conjugated with, contributes to the significance to this work. Focusing on the extrapolated results of over potentials, current densities and production rates of both hydrogen and oxygen throughout electrolysis is of utmost importance. Notably, CQDs exhibited low Tafel slopes (35–45 mV/dec), along with crucial traits such as stability and rapid electron transfer rates, affirming their potential as electrocatalysts. Among the various metal alloy nanoparticles investigated, suitable candidates for conjugation were identified. Collectively, the collated data suggests that a CQD/metal alloy nanoparticle conjugation could enhance the water splitting process for commercial applications, particularly in the underexplored realm of hydrogen production. However, it remains imperative to perform experimental procedures to substantiate this proposition when feasible.
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