材料科学
纳米纤维
纤维素
韧性
细菌纤维素
聚合物
复合材料
极限抗拉强度
纳米技术
复合数
化学工程
工程类
作者
Jie Wei,Suotang Jia,Jie Wei,Chao Ma,Ziqiang Shao
标识
DOI:10.1021/acsami.1c09653
摘要
Although humidity-responsive actuators serve as a promising candidate in smart wearables, artificial muscles, and biomimetic devices, most of them derived from synthetic polymers could not simultaneously achieve multifunctional properties. In this work, a cellulose nanofiber (CNF)-based film actuator with high mechanical properties, excellent Joule heating, and antibacterial capability is successfully constructed by integrating with Ti3C2Tx (MXene) and tannic acid (TA) via a vacuum-assisted filtration approach. Owing to the unique nacrelike structure and strong hydrogen bonds, the tensile strength and toughness of the composite film could reach 275.4 MPa and 10.2 MJ·m-3, respectively. Importantly, the hydrophilic nature of CNFs and alterable interlayer spacing of MXene nanosheets endow the composite film with sensitive humidity response and extraordinary stability (1000 cycles). With the assistance of MXene nanosheets and TA, the composite film could not only present outstanding Joule heating but also possess remarkable antibacterial properties against both Gram-negative Escherichia coli and Gram-positive Staphylococcus aureus. Benefiting from the above merits, the proof-of-concept smart garment is assembled by the as-prepared film and is capable of regulating humidity and temperature.
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