Graphene‐Enabled Superior and Tunable Photomechanical Actuation in Liquid Crystalline Elastomer Nanocomposites

Programmable photoactuation enabled by graphene: Graphene sheets aligned in liquid crystalline elastomers are capable of absorbing near-infrared light. They thereafter act as nanoheaters and provide thermally conductive pathways to trigger the nematic-to-isotropic transition of elastomers, leading to macroscopic mechanical deformation of nanocomposites. Large strain, high actuation force, high initial sensitivity, fast reversible response, and long cyclability are concurrently achieved in nanocomposites.