Engineering of Ultra‐Thin Layer of MIL‐125(Ti) Nanosheet\Zn‐Tetracarboxy‐Phthalocyanine S‐Scheme Heterojunction as Photocatalytic CO2 Reduction Catalyst

Metal-organic frameworks (MOFs) with ultrathin 2D structure have attracted remarkable attention in photocatalytic application owing to the accessibility of abundant active sites on the surface. But high charge recombination results in poor photocatalytic activity. Herein, the synthesis of ultrathin MIL-125(Ti) nanosheets is reported with a thickness of 1.3 nm through a simple chemical reaction route of precursor solution aging and subsequent solvothermal process for photocatalytic CO