Photoluminescent Properties of Erbium-Doped Aluminum Scandium Nitride Thin Films

材料科学 光致发光 兴奋剂 光电子学 光子学 激光器 氮化物 薄膜 氮化硅 光学 纳米技术 物理 图层(电子) 冶金
作者
Xingyan Zhao,Ziluo Xie,Huayou Liu,Huan Liu,Yuanmao Pu,Yang Qiu,Shaonan Zheng,Yaping Dan,Qize Zhong,Yuan Dong,Ting Hu
出处
期刊:ACS Photonics [American Chemical Society]
标识
DOI:10.1021/acsphotonics.4c01951
摘要

Scandium (Sc)-doped aluminum nitride (AlN) (Al1–xScxN) has attracted increasing attention in integrated photonics due to its remarkable piezoelectric, electro-optic, and acousto-optic properties. Erbium (Er)-doped Al1–xScxN presents promising opportunities for the development of high-gain integrated optical amplifiers and high-efficiency lasers in silicon photonic applications. However, research on the photoluminescent (PL) properties of Er-doped Al1–xScxN films remains limited. In this work, the PL properties of Er-doped Al1–xScxN films are investigated systematically across different Er and Sc concentrations. Strong PL emission at communication wavelengths was observed at room temperature. The PL intensity of the Er-doped Al0.904Sc0.096N sample is more than five times higher than that of the Er-doped AlN sample with the same Er doping concentration under identical excitation conditions. Additionally, the PL intensity of the Er-doped Al0.904Sc0.096N sample remained nearly constant as the temperature increases from 77 to 300 K, indicating a significantly suppressed thermal quenching effect. Notably, the 0.3% Er-doped Al0.904Sc0.096N sample exhibited a PL intensity up to 70 times higher than that of the commercially available 0.5%Er-doped lithium niobate on the insulator sample, demonstrating a strong potential for applications in integrated optical amplifiers and lasers on silicon photonic platforms.
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