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The planar chiral [2.2]paracyclophane (PCP) has garnered considerable attention due to its widespread applications. A chiral phosphoric acid catalyzed asymmetric reductive amination of pseudo ‐ para ‐diformyl [2.2]PCP was developed, allowing for access to a series of benzylamine‐containing 4,16‐disubstituted planar chiral [2.2]PCPs with good yields and high to perfect enantioselectivities. Diverse downstream transformations highlighted the value of current method. More details are discussed in the article by Wang et al . on pages 924—930. image