电催化剂
海水
电解质
材料科学
电化学
纳米材料
化学工程
分解水
可再生能源
纳米技术
催化作用
电极
化学
有机化学
光催化
海洋学
电气工程
地质学
工程类
物理化学
作者
Yingxue Du,Qichang Li,Mengzhen Liu,Dongzheng Liu,Weiping Xiao,Zhenyu Xiao,Zhenjiang Li,Yusuke Yamauchi,Sameh M. Osman,Zexing Wu,Lei Wang
标识
DOI:10.1016/j.cej.2023.146057
摘要
The search for promising methods of hydrogen production has led to the development of electrocatalytic overall seawater splitting. We have successfully prepared a highly efficient and durable electrocatalyst, Cu-based hollow nanotubes with rough surfaces coupled with chloridion-enriched environment on copper foam, through in-situ corrosive engineering and cation/anion exchange at room temperature. This innovative approach has resulted in an electrocatalyst with excellent electrochemical activity and stability in seawater electrolyte, which could potentially revolutionize the field of renewable energy. Remarkably, this electrocatalyst requires only a small voltage of 1.55 V to achieve a current density of 10 mA cm−2 in a tedious seawater electrolyte, with excellent stability at 200 mA cm−2 for 100 h. Our work provides a valuable avenue for increasing the active sites and corrosion resistance of synthesized nanomaterials, making them a viable option for renewable energy-related applications.
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