On the prospects of high-entropy organic A-site halide perovskites

values up to almost 0.08, resulting in one of the highest configurational entropies ever reported in A-site-only mixed HPs. The high-entropy HPs also showed band gaps of about 1.5 eV, decreased ionic transport, and remarkable stability compared to the unsubstituted composition. The results consolidate the potential of maximizing the configurational entropy as a design parameter in HPs.