Metal–Organic Frameworks: Molecular‐Scale Interface Engineering of Metal–Organic Frameworks toward Ion Transport Enables High‐Performance Solid Lithium Metal Battery (Adv. Funct. Mater. 50/2020)

In article number 2003945, Qi Zhang, Shaoming Huang, and co-workers develop a molecular-level interface engineering strategy with long-chain Lewis bases to optimize long-distance ion transport across interfaces in solid electrolytes consisting of metal-organic frameworks. The engineered solid electrolyte demonstrates single ion transport capability and higher ion conductivity and endows the solid-state battery with higher capacity and longer lifetime.