光电探测器
光电子学
异质结
材料科学
范德瓦尔斯力
灵敏度(控制系统)
宽禁带半导体
物理
电子工程
分子
量子力学
工程类
作者
Greg Sun,Wenjie Li,Peng Wan,Tong Xu,Yalin Zhai,Chongbiao Luan,Yang Zhou,Caixia Kan,Daning Shi,Mingming Jiang
摘要
High-fidelity quantitative detection in the solar-blind ultraviolet regime is essential for radiation-hardened optical systems and secure communications. This study demonstrates a pioneering self-powered ultraviolet photodetector utilizing an engineered CsCu2I3/AlGaN van der Waals heterojunction (vdWh) architecture, enabling high-precision light irradiance measurement. Through strategic integration of size-controlled platinum nanoparticles (PtNPs) that induce localized surface plasmon resonances enhancement, the optimized device achieves remarkable performance metrics at zero bias: a photoresponsivity of 200 mA/W, a specific detectivity of 1.65 × 1012 Jones as well as ultrafast response speed with rise/fall times of 400/540 μs under 254 nm illumination, surpassing the majority of its competitors. The unencapsulated detector exhibits robust thermal-humidity stability under ambient conditions, demonstrating exceptional reliability. A prototype light-intensity monitoring system, integrating this PtNPs@CsCu2I3/AlGaN vdWh detector with customized signal processing circuitry, demonstrates exceptional measurement accuracy with absolute error < 5.0 μ W/cm2 and relative error < 5.0%, respectively. This work develops high-performance solar-blind ultraviolet photodetectors using eco-friendly lead-free perovskites with tailored interfaces, and establishes an integration framework bridging these devices to deep-ultraviolet photonics and radiation-resistant applications.
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