Comment on amt-2022-48

环境科学 化石燃料 放射性碳年代测定 反演(地质) 温室气体 碳循环 大气科学 遥感 生态系统 地质学 海洋学 化学 生态学 地貌学 古生物学 有机化学 构造盆地 生物
标识
DOI:10.5194/amt-2022-48-rc2
摘要

Abstract. Various satellite imagers of the vertically integrated column of carbon dioxide (XCO2) are under development to enhance the capabilities for the monitoring of the fossil fuel (FF) CO2 emissions. XCO2 images can be used to detect plumes from cities and large industrial plants, and to quantify the corresponding emissions using atmospheric inversions techniques. However, this potential and the ability to catch the signal from more diffuse FF CO2 sources can be hampered by the mix between these FF signals and a background signal from other types of CO2 surface fluxes, and in particular of biogenic CO2 fluxes. The deployment of dense ground-based air-sampling networks for CO2 and radiocarbon (14CO2) could complement the spaceborne imagery by supporting the separation between the fossil fuel and biogenic or biofuel (BF) CO2 signals. We evaluate this potential complementarity with a high resolution analytical inversion system focused on Northern France, Western Germany, Belgium, Luxembourg and a part of the Netherlands, and with pseudo-data experiments. The inversion system controls the FF and BF emissions from the large urban areas and plants, in addition to regional budgets of more diffuse emissions or of biogenic fluxes (NEE, Net Ecosystem Exchange), at an hourly scale over a whole day. The system assimilates pseudo data from a single track of a 300-km swath XCO2 imager at 2 km resolution and from surface ground-based CO2 and/or 14CO2 networks. It represents the diversity of 14CO2 sources and sinks and not just the dilution of radiocarbon-free FF CO2 emissions. The uncertainty in the resulting FF CO2 emissions at local (urban area/ plant) to regional scales is directly derived and used to assess the potential of the different combinations of observation systems. The assimilation of satellite observations yield estimates of the morning regional emissions with an uncertainty down to 10 % (1 sigma) in the satellite field of view, from an assumed uncertainty of 15 % in the prior estimates. However, it does not provide direct information about emissions outside the satellite field of view and neither about afternoon or nighttime emissions. The co-assimilation of 14CO2 and CO2 data lead to a further reduction of the uncertainty in the estimates of FF emissions. However, this further reduction is significant only in administrative regions with three or more 14CO2 and CO2 sampling sites. The uncertainty in the estimates of 1-day emission in North Rhine-Westphalia, a region with three sampling sites, decreases from 8 to 6.6 % when assimilating the in situ 14CO2 and CO2 data in addition to the satellite data. Furthermore, this new decrease appears to be larger when the ground stations are close to large FF emission areas, providing an additional direct constraint for the estimate of these sources rather than supporting the characterization of the background signal from the NEE and its separation from that of the FF emissions.

科研通智能强力驱动
Strongly Powered by AbleSci AI
科研通是完全免费的文献互助平台,具备全网最快的应助速度,最高的求助完成率。 对每一个文献求助,科研通都将尽心尽力,给求助人一个满意的交代。
实时播报
罗远远完成签到,获得积分10
刚刚
Hanny完成签到 ,获得积分10
刚刚
执刀手完成签到 ,获得积分10
1秒前
维E真发布了新的文献求助10
1秒前
1秒前
小马甲应助个性的身影采纳,获得10
3秒前
3秒前
5秒前
若一发布了新的文献求助10
5秒前
华仔应助贾硕士采纳,获得10
6秒前
qqct完成签到,获得积分10
6秒前
71发布了新的文献求助10
6秒前
玉渊潭完成签到,获得积分10
7秒前
7秒前
Alice001完成签到 ,获得积分10
7秒前
8秒前
ychope完成签到,获得积分10
8秒前
8秒前
YJDDDF应助阔达尔云采纳,获得30
9秒前
端庄的静曼完成签到,获得积分10
9秒前
9秒前
Hello应助纯牛马打工人采纳,获得10
10秒前
肥猫啊平发布了新的文献求助10
10秒前
研友_VZG7GZ应助Leo采纳,获得30
11秒前
cz完成签到 ,获得积分10
12秒前
李健应助辛勤的喉采纳,获得10
12秒前
大个应助Yanzhang0000采纳,获得10
13秒前
蔡宇滔发布了新的文献求助10
13秒前
DWH发布了新的文献求助10
13秒前
Jasper应助nanjiluotuo11采纳,获得10
13秒前
宫宛儿发布了新的文献求助10
14秒前
不吃辣活不了完成签到,获得积分10
14秒前
15秒前
木子完成签到,获得积分10
15秒前
黄小豆完成签到,获得积分10
17秒前
静坐听雨萧完成签到 ,获得积分10
17秒前
17秒前
MANTISYAO发布了新的文献求助10
18秒前
Yanzhang0000完成签到,获得积分10
18秒前
19秒前
高分求助中
(应助此贴封号)【重要!!请各用户(尤其是新用户)详细阅读】【科研通的精品贴汇总】 10000
Reducing Compassion Fatigue, Secondary Traumatic Stress and Burnout 600
China Pluperfect I: Epistemology of Past and Outside in Chinese Art 520
Matrix Methods in Data Mining and Pattern Recognition Second Edition 510
Mammalian Synthetic Biology 500
Auslegungsgeschichte 500
Cosmos as Art Object: Studies in Plato's Timaeus and Other Dialogues 500
热门求助领域 (近24小时)
化学 材料科学 医学 生物 纳米技术 工程类 有机化学 化学工程 生物化学 计算机科学 内科学 物理 复合材料 催化作用 细胞生物学 无机化学 光电子学 物理化学 电极 基因
热门帖子
关注 科研通微信公众号,转发送积分 7638150
求助须知:如何正确求助?哪些是违规求助? 9211446
关于积分的说明 19758767
捐赠科研通 7205055
什么是DOI,文献DOI怎么找? 3275778
关于科研通互助平台的介绍 2437416
邀请新用户注册赠送积分活动 2272986