In parity-time-symmetric (PT-symmetric) Hamiltonian theory, the optimal evolution time can be reduced drastically and can even be zero. In this article, we report our experimental simulation of the fast evolution of a PT-symmetric Hamiltonian in a nuclear magnetic resonance quantum system. The experimental results demonstrate that the PT-symmetric Hamiltonian system can indeed evolve much faster than the quantum system, and the evolution time can be arbitrarily close to zero.