蒸发器
材料科学
蒸发
海水淡化
制作
碳纳米管
太阳能
太阳能淡化
纤维素
吸收(声学)
化学工程
纳米技术
海水
工艺工程
纳米晶
可再生能源
电阻率和电导率
光电子学
能量转换效率
光伏系统
余热
太阳能蒸馏器
碳纤维
电导率
电流(流体)
纳米颗粒
作者
Ping Xie,Chuanliang Chen,Ke Tian,Minhan Cheng,Qianyang Li,Hua Deng
出处
期刊:Langmuir
[American Chemical Society]
日期:2025-10-17
卷期号:41 (42): 28905-28915
标识
DOI:10.1021/acs.langmuir.5c04689
摘要
The development of efficient and sustainable solar-driven water evaporation systems is crucial for mitigating global water scarcity. However, the intermittent nature of solar radiation presents a major challenge for achieving continuous steam generation under all conditions. Most current fabrication methods for solar evaporators lack scalability, flexibility, and environmental compatibility. Herein, we present a scalable-fabricated solar evaporator with a gradient-heating design, constructed from PET/CNT/PDA/CNC@CuS composites for continuous steam generation. This device synergistically utilizes solar illumination and electrical heating, enabled by the strong broadband light absorption and excellent electrical conductivity imparted by a two-step spray-coating of carbon nanotubes (CNT) and CuS-decorated cellulose nanocrystals (CNC@CuS). Cellulose nanocrystals (CNC) are used to uniformly load commercial CuS powder onto CNT/PDA-coated PET fabric via electrostatic and hydrogen-bond interactions. Synergistic effect combining 1-sun illumination and 5 V input elevates the evaporation rate to 5.49 kg m-2 h-1, with temperature surpassing individual modes by 6.8 °C (light-only) and 4.2 °C (electricity-only). The evaporator demonstrates remarkable salt tolerance, maintaining 5.3 kg m-2 h-1 in 3.5 wt % NaCl (1-sun and 5 V) and 2.3 kg m-2 h-1 (only 5 V), with no performance decline over 7 days. Furthermore, the CNC@CuS coatings also impart intrinsic antibacterial and UV-shielding properties. This study provides a promising approach for environmentally friendly, efficient, and all-weather seawater desalination.
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