光催化
材料科学
碳纤维
多孔性
化学工程
纳米技术
复合数
产量(工程)
催化作用
复合材料
化学
有机化学
工程类
作者
Lichun Deng,Yuanli Li,Zhenghan Zhang,Yihong Zhang,Jiaxing Zhong,Can Zhang,Hang Zhang,Chunqiang Zhuang
出处
期刊:ACS applied nano materials
[American Chemical Society]
日期:2023-08-29
标识
DOI:10.1021/acsanm.3c02980
摘要
Efficient charge separation is one of the critical issues for the design of photocatalytic systems. The physical mixing of photocatalysts and cocatalysts to prepare photocatalytic systems usually leads to a high interfacial resistance, which is not beneficial to efficient charge separation. Here, we report the in situ construction of photocatalytic systems by directly growing CdS nanosheets on porous carbon aerogels (CA) to obtain photocatalytic systems with compact interfacial contact. The photocatalytic H2 yield of the optimized CdS@CA composite is ∼27.3 mmol/g, obviously higher than that of CdS nanosheets (∼11.4 mmol/g). Electrochemical and spectroscopic methods demonstrate that the incorporation of carbon aerogels with CdS nanosheets can efficiently inhibit the recombination of photo-generated electrons and holes, thus achieving highly improved photocatalytic H2 production.
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