光催化
材料科学
废水
纳米片
降级(电信)
罗丹明B
化学工程
光热治疗
蒸发
污水处理
氧化物
无机化学
环境工程
冶金
纳米技术
化学
环境科学
催化作用
物理
工程类
热力学
电信
生物化学
计算机科学
作者
Mengyu Guo,Baohua Yuan,Ying Sui,Yu X,Jing Dong,Lixia Yang,Liangjiu Bai,Huawei Yang,Daming Wei,Wenxiang Wang,Na Yang
标识
DOI:10.1016/j.jcis.2022.11.015
摘要
Integrating advanced technologies into solar-driven water evaporation is gradually considered as a clean and sustainable way to acquire freshwater from saline or wastewater. In this study, thin molybdenum sulfide nanosheet arrays (MoS2 NSAs) modified by tungsten oxide nanoparticles (WO3) were designed. The as-prepared solar absorber could purify water and accomplish photocatalytic degradation of dyes that existed in bulk water via solar-driven water evaporation. Compared with bare MoS2 NSAs, the modification of WO3 enhanced the separation of electrons and holes within the solar absorber, resulting in the improvement of photocatalytic efficiency. The net evaporation rate of the solar absorber reached 0.97 kg m-2h-1 and the degradation rate constant of rhodamine B (RhB) reached 0.101 min-1 under 1 sun. This study successfully combined photothermal conversion and photocatalytic technologies and provided a new method for the treatment of dye wastewater with zero wastewater discharge.
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