Achieving excellent physico-mechanical properties of Cu matrix composites by incorporating a low content of a three-dimensional graphene network

In-depth investigation of the distribution form of the reinforcement and associated mechanisms has great significance for fabricating highly strengthened and conductive Cu matrix composites. The three-dimensional graphene (3DG) network can withstand more strain due to its large specific surface area, and provides interlinked high-speed conductive paths within the composites. In this study, we propose a feasible method to fabricate 3DG-reinforced Cu matrix composites; here, the Cu foam serves as the initial substrate during the chemical vapour deposition (CVD) process and as the matrix of the composites. Through constructing an ideal 3DG network, the graphene content is approximately 0.28 vol%, and a remarkable 230 % improvement in the ultimate tensile strength (418 MPa) with a high electrical conductivity (97.02 %IACS) is obtained in the composite. The continuous high-quality 3DG network is conducive for achieving excellent physico-mechanical properties of the composites, and the enhanced efficiency is superior. A new concept of fabricating Cu matrix composites was proposed for future research.